Myron Healey

John Dillinger (archive footage)

Paul Dubov

Alvin Karpis

Sam Edwards

Fred Barker

Richard Crane

Homer Van Meter

Lyle Talbot

Dr. William Guellfe, Plastic Surgeon

Jeanne Carmen

Paula

Tamar Cooper

Bonnie Parker

Baynes Barron

Clyde Barrow

Doug Wilson

Charles Arthur 'Pretty Boy' Floyd

Jim Davis

Police Captain Stewart / Narrator

Sydney Mason

Lieutenant Bill Baxter

Lash LaRue

'Doc' Barker

Ralph Moody

Arthur 'Pa' Barker

Ann Morriss

Mildred Jaunce - The Lady in Red

Aline Towne

Shirley, Girl with Karpis

Regina Gleason

Hope

Jeanne Bates

Mrs. Ross Baxter

Jean Harvey

'Ma' Barker (archive footage)

Helen Van Tuyl

Texas Lady Governor (archive footage)