Burgess Meredith

Dr. Diabolo (Framing Story)

Jack Palance

Ronald Wyatt (segment 4 "The Man Who Collected Poe")

Beverly Adams

Carla Hayes (segment 2 "Terror Over Hollywood")

Peter Cushing

Lancelot Canning (segment 4 "The Man Who Collected Poe")

Maurice Denham

Uncle Roger (segment 1 "Enoch")

Barbara Ewing

Dorothy Endicott (segment 3 "Mr. Steinway")

Michael Bryant

Colin Williams (segment 1 "Enoch")

John Standing

Leo Winston (segment 3 "Mr. Steinway")

Robert Hutton

Bruce Benton (segment 2 "Terror Over Hollywood")

John Phillips

Eddie Storm (segment 2 "Terror Over Hollywood")

Michael Ripper

Gordon Roberts (Framing Story)

Bernard Kay

Dr. Heim (segment 2 "Terror Over Hollywood")

Catherine Finn

Nurse Parker (segment 1 "Enoch")

Ursula Howells

Miss Maxine Chambers (segment 3 "Mr. Steinway")

David Bauer

Mike Charles (segment 2 "Terror Over Hollywood")

Niall MacGinnis

Dr. Silversmith (segment 1 "Enoch")

Hedger Wallace

Edgar Allan Poe(segment "4 "The Man Who Collected Poe"")

Clytie Jessop

Atropos, Goddess of Destiny